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Position: Home > issue > February 28, 2021 Volume 2, Issue 1
Controllable Generation of Reactive Oxygen Species on Cyano-Group-Modified Carbon Nitride for Selective Epoxidation of Styrene
Category: Report
Author: Hao Tan, Peng Kong, Riguang Zhang, Mengting Gao, Meixian Liu, Xianmo Gu, Weifeng Liu, Zhanfeng Zheng

2.jpg

Graphical Abstract


The controlled generation of reactive oxygen species (ROS) to selectively epoxidize styrene is a grand challenge. Herein, cyano-group-modified carbon nitrides (CNCYx and CN-Ty) are prepared, and the catalysts show better performance in regulating ROS and producing styrene oxide than the cyano-free sample. The in situ diffuse reflectance infrared and density functional theory calculation results reveal that the cyano group acts as the adsorption and activation site of oxygen. X-ray photoelectron spectroscopy and NMR spectrum results confirm that the cyano group bonds with the intact heptazine ring.





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