CO2-mediated conversion of physical pressure into chemical pressure to realize lattice strain
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PUBLIC SUMMARY
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Supercritical CO2 mediates the conversion of physical pressure into chemical pressure induced lattice strain.
Lattice strain effectively modulates the coupling between spins, charges and orbitals in materials.
Lattice strain brings some novel physical phenomena.
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ABSTRACT
Lattice strains often lead to novel phenomena, and they are used in a variety of applications, such as thermoelectricity, ferroelectricity, ferromagnetic, skyrmion and superconductivity. In this paper, we briefly summarize the novel phenomena brought about by lattice strain. An efficient method to realize lattice strain using supercritical CO2 (SC CO2) is proposed. When CO2 molecules shuttle through the confined space of the crystal structure, it can generate huge energy subsequently. Specifically, CO2 carries MPa-level external physical pressure inside the crystal structure, forming localized defects or phase transitions. This alters the original chemical coordination environment and generates internal chemical pressures up to the GPa level. The crystal is stripped from three-dimensional to two-dimensional under high pressure, and lattice strain is realized at the same time. This work will provide new insights into the realization of lattice strain and give valuable guidance to broaden its application. -
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REFERENCES
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Gao B. and Xu Q. (2024). CO2-mediated conversion of physical pressure into chemical pressure to realize lattice strain. The Innovation Materials 2(3): 100083. https://doi.org/10.59717/j.xinn-mater.2024.100083
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Gao B. and Xu Q. (2024). CO2-mediated conversion of physical pressure into chemical pressure to realize lattice strain. The Innovation Materials 2(3): 100083. https://doi.org/10.59717/j.xinn-mater.2024.100083
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Content
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Figure 1.
SC CO2 acts on materials
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Figure 2.
Improving the performance of thermoelectric materials and modules through entropy engineering
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Figure 3.
Strain-induced ferroelectricity in BaTiO3 and PbTiO3
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Figure 4.
Structural and electronic state characterizations of the (LmSn) superlattices
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Figure 5.
Generation of lattice strain
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Figure 6.
Lattice strain under the action of SC CO2
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Figure 7.
Strain-induced ferromagnetism of SrTiO3 and BiFeO3
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Figure 8.
Microstructural characterization of nanosheets
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Figure 9.
Luminescence Properties of BaTiO3 and SrTiO3
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Figure 10.
Strain-induced catalytic properties
