Precise design of chiral-polar hybrid perovskites toward efficient self-powered full-stokes photodetection

Huajie Wu; Zhijin Xu; Xin Dong; Lei Wang; Jing Liang; Tianqi Chen; Xiaoqi Li; Lina Li; Junhua Luo

doi:10.59717/j.xinn-mater.2024.100084

The Innovation Materials > 2024 Vol. 2 > No. 3 > 100084

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Precise design of chiral-polar hybrid perovskites toward efficient self-powered full-stokes photodetection

1.
State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou 350002, China
2.
College of Chemistry and Materials Science Fujian Normal University, Fuzhou 350007, China
3.
University of Chinese Academy of Sciences, Beijing 100049, China

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Corresponding authors: lilina@fjirsm.ac.cn (L. L.)
Received Date: April 30, 2024

Accepted Date: July 29, 2024

Published Online: July 30, 2024

The Innovation Materials 2(3), https://doi.org/10.59717/j.xinn-mater.2024.100084 | Cite this article

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PUBLIC SUMMARY

PUBLIC SUMMARY
1. Two novel chiral-polar hybrid perovskites were successfully synthesized.
  
  A self-powered full-Stokes photodetection with the Stokes parameter averaging error of less than 0.08 was acquired.
  
  Provides new insights into the design of materials for high-performance multipolarization state photodetection.

ABSTRACT

ABSTRACT

Full-Stokes polarimeters can efficiently discriminate the multipolarization of lights, showing great potential in fields of medical science, military and optoelectronics. However, most of the current full-Stokes polarimeters are limited by complex optical devices and low detection accuracy of Stokes vectors, which impeded their practical optoelectronic application. In this work, we successfully designed two novel chiral-polar hybrid perovskites, ((R)-β-MPA)PAPbI₄ and ((S)-β-MPA)PAPbI₄ (R-1 and S-1, MPA = methylphenethylamine and PA = propylamine), which show distinctive bulk photovoltaic effect (BPVE). The BPVE enables efficient self-driven detection of linearly and circularly polarized light (LPL and CPL, respectively) in a single-crystal device of R-1. Such detection possesses high LPL sensitivity with a polarization ratio reaching 1.52 and CPL distinguishability reaching 0.4, achieving highly accurate full-Stokes polarization detection with the Stokes parameter averaging error of less than 0.08. To the best of our knowledge, this is the first report on chiral hybrid perovskite realizing self-powered full-Stokes photodetection based on BPVE. These results provide new insights into the design of chiral materials for high-performance multipolarization photodetection.

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Wu H., Xu Z., Dong X., et al., (2024). Precise design of chiral-polar hybrid perovskites toward efficient self-powered full-stokes photodetection. The Innovation Materials 2(3): 100084. https://doi.org/10.59717/j.xinn-mater.2024.100084

Wu H., Xu Z., Dong X., et al., (2024). Precise design of chiral-polar hybrid perovskites toward efficient self-powered full-stokes photodetection. The Innovation Materials 2(3): 100084. https://doi.org/10.59717/j.xinn-mater.2024.100084

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