Universal Taxol molecular binding engineering in dual-polarity MoS2 photodetector

Yongkang Jiang; YuSheng Xie; Qiming Pan; Jinping Li; Qi Zhan; Yujie Sun; JinShan Wang; Yang Ren; Xinghong Wang; Kenan Zhang; Feng Qiu

doi:10.59717/j.xinn-mater.2026.100191

The Innovation Materials > 2026 Vol. 4 > No. 1 > 100191

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Universal Taxol molecular binding engineering in dual-polarity MoS₂ photodetector

1.
National Center for International Joint Research of Photoelectric Energy Materials and Application, Yunnan Key Laboratory of Electromagnetic Materials and Devices, School of Materials and Energy, Yunnan University, Kunming 650500, China
2.
School of Physics and Astronomy, Yunnan University, Kunming 650500, China
3.
Yunnan Institute of Microbiology, Yunnan University, Kunming 650500, China
4.
Department of Electrical Engineering and Computer Science, Massachusetts Institute of Technology, Cambridge 02139, USA
5.
These authors contributed equally

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Corresponding authors: fengqiu@ynu.edu.cn (F.Q.); reny@ynu.edu.cn (Y.R.); kenzhang@mit.edu (K.Z.)
Received Date: June 11, 2025

Accepted Date: January 07, 2026

Published Online: January 16, 2026

The Innovation Materials 4(1), https://doi.org/10.59717/j.xinn-mater.2026.100191 | Cite this article

GRAPHICAL ABSTRACT

GRAPHICAL ABSTRACT

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PUBLIC SUMMARY

PUBLIC SUMMARY
1. Taxol molecules hold considerable potential for enhancing the optoelectronic performance of 2D materials.
  
  Taxol can effectively passivate the interfacial defects of MoS₂ while preserving its crystalline integrity.
  
  Establishing interfacial Mo-O bonding pathways enables directional electron transfer.
  
  Taxol modification strategy enables increased carrier mobility and reduced electronic noise.

ABSTRACT

ABSTRACT

Intrinsic defects in two-dimensional (2D) atomic crystals impose severe constraints on carrier utilization through defect-induced trapping and recombination. While surface modification and mobility recovery strategies have been widely explored, the development of a universal defect mitigation protocol remains unresolved. Here, we introduce a molecular passivation strategy in which Taxol molecules, via their hydroxyl radicals, repair intrinsic sulfur vacancies in monolayer MoS₂, thereby markedly accelerating carrier transport dynamics. The Taxol framework not only modulates the electronic structure of n-type MoS₂ lattices but also shows compatibility with p-type MoS₂ configurations, enabling robust interfacial unit cell binding. Following modification, both n- and p-type MoS₂ exhibit acoustic phonon-limited mobilities enhanced and more than an order of magnitude for p-type conuterpart. This universal lattice-reconstruction strategy further suppresses noise power by up to six orders of magnitude and restrain interface state, while achieving a responsivity above 200 A W⁻¹ and specific detectivity exceeding 1.0 × 10¹² Jones — representing an improvement of four orders of magnitude. Complementary theoretical calculations confirm that Taxol-mediated coordination effectively passivates sulfur vacancies and optimizes charge transport. These findings establish a universal molecular coordination protocol to mitigate defect-related noise currents and boost detection sensitivity, advancing the performance of 2D photodetectors for next-generation optoelectronic and biosensing applications.
- Taxol molecule /
- Universal binding protocol /
- Surface modification /
- Dual-polarity MoS₂ /
- Two-dimensional photodetector

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Jiang Y., Xie Y., Pan Q., et al. (2026). Universal Taxol molecular binding engineering in dual-polarity MoS2 photodetector. The Innovation Materials 4:100191. https://doi.org/10.59717/j.xinn-mater.2026.100191

Jiang Y., Xie Y., Pan Q., et al. (2026). Universal Taxol molecular binding engineering in dual-polarity MoS₂ photodetector. The Innovation Materials 4:100191. https://doi.org/10.59717/j.xinn-mater.2026.100191

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